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TABI specifically for the interaction between two dielectric spheres, with multiple charges inside each sphere

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TABI-2spheres

This repo provides a version of the TABI code for the case of two dielectric spheres with multiple charges inside each sphere and surrounded by ionic solvent. The code solves the linear Poisson-Boltzmann equation for the surface potential using the Juffer et al. (1991) integral formulation and a boundary element method. The spheres are discretized using the icosahedral triangulation. The code is written in Fortran.

how to run it

Type make, then run the executable file "./tabipb.exe".

input files

The TABI parameters are in file usrdata.in and the data for the two spheres is in folder 2sphere_data; the sample data in this folder is from Table 1 in Zhou (1993).

input: usrdata.in (parameters for TABI)

epsp: dielectric constant inside spheres; default is 4
epsw: dielectric constant of solvent; default is 78.5
bulk_strength: ionic concentration strength (M); default is 0.16
den: integer number of refinement levels on each sphere; default is 3
order: treecode multipole expansion order; default is 3
maxparnode: maximum particles per leaf for octree; default is 500
mac: multipole acceptance criterion for treecode; default is 0.5

input: 2sphere_data (data for 2 spheres)

This folder contains two files, oneb_sph1.pqr, oneb_sph2.pqr, with the data describing the two spheres. Each line in the files corresponds to a charge. There are 5 columns for each line containing information about the charge as follows. All lengths are in units of angstroms and charges are in units of e.

column 1: x-coordinate of charge
column 2: y-coordinate of charge
column 3: z-coordinate of charge
column 4: charge value of charge
column 5: radius of sphere enclosing the charge

We assume each sphere has a central charge, which is the first line of each pqr file. Starting from the second line, we list the off-center charges. If there is no central charge, then set the charge value of the first line to zero.

output file 1: energy.dat

This gives the total electrostatic free energy (Coulomb and solvation) of the 2-sphere system in units of kcal/mol.

To find the interaction energy, compute and subtract from the above value the total electrostatic free energy for the 2-sphere system when the spheres are far from each other, say a few Debye lengths. This just needs to be calculated once.

output file 2: surface_potential.dat

This gives the surface potential values in a format suitable for plotting with VMD.

The 1st line gives the number of vertices and the number of triangles for the entire 2-sphere system.

The next lines gives infomation about each vertex (index of vertex, xyz coordinates of vertex, normal vector at vertex, surface potential at vertex [kcal/mol/ec], surface potential normal derivative at vertex [kcal/mol/ec/Å].

The next lines give the connectivity data for the surface triangulation.

References

W.H. Geng, R. Krasny, A treecode-accelerated boundary integral Poisson-Boltzmann solver for electrostatics of solvated biomolecules, J. Comput. Phys., 247, 62-78 (2013).

A.H. Juffer, E.F.F. Botta, B.A.M. van Keulen, A. van der Ploeg, H.J.C. Berendsen, The electric potential of a macromolecule in a solvent: A fundamental approach, J. Comput. Phys., 97, 144-171 (1991).

H.-X. Zhou, Brownian dynamics study of the influences of electrostatic interaction and diffusion on protein-protein association kinetics, Biophys. J., 64, 1711-1726 (1993).

This work was funded by National Science Foundation grants DMS-1418966 and DMS-1819094.

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TABI specifically for the interaction between two dielectric spheres, with multiple charges inside each sphere

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